By Georgia S. Lemen, John P. Wolfe (auth.), Marc Taillefer, Dawei Ma (eds.)
Palladium-Catalyzed sp2C–N Bond Forming Reactions: fresh advancements and functions. Metal-catalyzed C(sp2)-N bond formation.- fresh advancements in Recyclable Copper Catalyst structures for C−N Bond Forming Cross-Coupling Reactions utilizing Aryl Halides and Arylboronic Acids. meeting of N-containing heterocycles through Pd and Cu-catalyzed C-N bond formation reactions. Copper-Catalyzed C(aryl)-N Bond Formation.
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Extra info for Amination and Formation of sp2 C-N Bonds
Urgaonkar S, Verkade JG (2004) J Org Chem 69:9135–9142 79. Urgaonkar S, Verkade JG (2004) Adv Synth Catal 346:611–616 80. Reddy CV, Kingston JV, Verkade JG (2008) J Org Chem 73:3047–3062 81. Ackerman L (2006) Synthesis 1557–1571 82. Ackermann L (2007) Synlett 507–526 83. Ackermann L, Born R (2005) Angew Chem Int Ed 44:2444–2447 84. Anderson KW, Tundel RE, Ikawa T, Altman RA, Buchwald SL (2006) Angew Chem Int Ed 45:6523–6527 85. Tundel RE, Anderson KW, Buchwald SL (2006) J Org Chem 71:430–433 86.
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67). 2 Br t-BuNH2 Pd(OAc)2 (2 mol %) IPr•HCl (4 mol %) NaOtBu, toluene 110 °C 96% t-Bu t-Bu H N H N N H N H t-Bu t-Bu ð67Þ Synthesis of Azacalixarenes, Aza-Crowns, Porphryins, and Related Compounds Palladium-catalyzed N-arylation reactions have been employed in the synthesis or derivatization of a number of nitrogen-containing macrocycles, including azacalixarenes , aza-crown ethers , aza-cyclophanes [375, 376], and porphryins [377–379]. For example, Wang and coworkers have prepared azacalixarenes 56 that are capable of binding fullerenes using a cyclocondensation of N,N0 -dimethyl-1,3-phenylenediamine with dibromide 55 (Eq.
Amination and Formation of sp2 C-N Bonds by Georgia S. Lemen, John P. Wolfe (auth.), Marc Taillefer, Dawei Ma (eds.)